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Of the two options you mention, I'd give RememberTheMilk a go.

The RTM web interface is great for adding tasks from any machine you are on and you can also email tasks. If you take up their pro option, then they have a great iPhone client.

I'm using OmniFocus on the iPhone and iPad at the moment as I used to use it when I was using a Mac (I now work in a PC environment) and thought it was great. RTM don't yet have an iPad app, otherwise I'd still be with them.

I'm really missing the ability to add tasks via email and the browser, so I may be heading back to RTM even though the OmniFocus iPad app is pretty good. RTM also integrates (in a basic form) with Google Calendar.

If you go with Toodledo, try Taska as your iPad as it syncs and has a nice clean GTD interface.

rgds/alex