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Nope. That was the crux of the problem: I mistakenly assumed that the Quick Entry would be populated even if text wasn't selected. For example, if I am browsing a webpage and invoke the Quick Entry, I would expect OmniFocus to enter the title and URL of the webpage in the note when I don't have any text specifically selected. Or if I am looking at an e-mail in Mail, I would expect OmniFocus to enter the subject of and a link to the e-mail in the note when I don't have any text specifically selected.

So, all in all, it works, just not like I was expecting (or hoping for).

Thanks for your help though.